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Identification of gallotannins and ellagitannins in aged wine spirits: A new perspective using alternative ageing technology and high-resolution mass spectrometry

2022Journal article Open access
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dc.contributor.authorFernandes, Tiago A.
dc.contributor.authorAntunes, Alexandra M.M.
dc.contributor.authorCaldeira, Ilda
dc.contributor.authorAnjos, Ofélia
dc.contributor.authorFreitas, Victor
dc.contributor.authorFargeton, Laurent
dc.contributor.authorBoissier, Benjamin
dc.contributor.authorCatarino, Sofia
dc.contributor.authorCanas, Sara
dc.date.accessioned2022-07-18T09:05:17Z
dc.date.available2023-07-18T00:30:27Z
dc.date.issued2022
dc.description.abstractThis research was focused on identifying gallotannins and ellagitannins degradation pathways to better understand their behavior in complex media such as wine spirits (WS). A WS was aged with chestnut wood staves with three levels of micro-oxygenation, nitrogen, and using wooden barrels. Gallotannins and ellagitannins were identified by LC-ESI-HRMS/MS using a Q-TOF in samples collected at 8, 21, 60, 180, 270, and 365 days of ageing, allowed comparing their relative abundances according to the ageing technology. It was established for the first time, the importance of oxygen in gallotannins and ellagitannins formation/degradation pathways in WS and shading light into the explanation for the steady increase of gallic and ellagic acid contents on WS during ageing. The results also highlighted the presence of penta-O-galloyl-β-D-glucose, tetra-O-galloyl-β-D-glucose, tri- O-galloyl-β-D-glucose, di-O-galloyl-β-D-glucose, and mono-O-galloyl-β-D-glucose, 2,3-(S)-hexahydroxydiphenoyl- β-D-glucose, pedunculagin, isomers vescalagin/castalagin and two products stemming from ethanol-promoted oxidation of castalagin/vescalagin and vescalin/castalin, in the composition WS aged with chestnut woodpt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.citation2. Fernandes, T.A.; Antunes, A.M.M.; Caldeira, I.; Anjos, O.; de Freitas, V.; Fargeton, L.; Boissier, B.; Catarino, S.; Canas, S. Identification of Gallotannins and Ellagitannins in Aged Wine Spirits: A New Perspective Using Alternative Ageing Technology and High-Resolution Mass Spectrometry. Food Chem. 2022, 382, 132322pt_PT
dc.identifier.doihttps://doi.org/10.1016/j.foodchem.2022.132322pt_PT
dc.identifier.urihttp://hdl.handle.net/10400.5/24890
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherElsevierpt_PT
dc.relationNot Available
dc.relationForest Research Centre
dc.subjectageing wine spiritpt_PT
dc.subjecthydrolysable tanninspt_PT
dc.subjectmicro-oxygenationpt_PT
dc.subjectchestnutpt_PT
dc.subjectmass spectrometrypt_PT
dc.titleIdentification of gallotannins and ellagitannins in aged wine spirits: A new perspective using alternative ageing technology and high-resolution mass spectrometrypt_PT
dc.typejournal article
dspace.entity.typePublication
oaire.awardTitleNot Available
oaire.awardTitleForest Research Centre
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/9471 - RIDTI/PTDC%2FOCE-ETA%2F27819%2F2017/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/DL 57%2F2016/DL 57%2F2016%2FCP1382%2FCT0025/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F00239%2F2020/PT
oaire.citation.titleFood Chemistrypt_PT
oaire.fundingStream9471 - RIDTI
oaire.fundingStreamDL 57/2016
oaire.fundingStream6817 - DCRRNI ID
person.familyNameCatarino
person.givenNameSofia
person.identifier.ciencia-id7212-C53B-0F02
person.identifier.orcid0000-0002-6223-4377
person.identifier.ridD-2752-2013
person.identifier.scopus-author-id8354919700
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
rcaap.rightsopenAccesspt_PT
rcaap.typearticlept_PT
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relation.isAuthorOfPublication.latestForDiscovery067dca13-5a43-4bcb-b789-69cf0a5567c3
relation.isProjectOfPublication627882e1-519b-44d6-b886-3b92ca218701
relation.isProjectOfPublicationcd7df150-192b-4f82-825f-7895ad9ae890
relation.isProjectOfPublication56bd0ae9-f8da-4344-b9a2-f633d4f68b89
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